We have used the melt-assisted wetting of porous alumina templates to fabricate vertical nanorod arrays of P3HT and PCBM having core–shell nanostructures for application in polymer solar cells. The C-AFM current images revealed the difference of charge transport behavior of the core and shell moieties. As a result of superior carrier transport, the internal and external quantum efficiencies of these core/shell nanorod inverted solar cells were both higher than those of the corresponding
conventional inverted BHJ device. The optimized nanorod array structure had a high hole mobilitythat was over one order magnitude greater than that of the conventional BHJ structure; the corresponding device displayed more efficient carrier transport, which contributed to a higher short-circuit current density and PCE, relative to those of the conventional device. Furthermore, this approach is also applied for TiO2
nanorod/P3HT rod array device for solar cell application.
The development of novel materials for solar cell application, we have used Grignard metathesis polymerization to prepare a series of thiophene-based
copolymers through conjugation with electron-withdrawing 1,3,4-oxadiazole moieties in the polymer side chains. The photocurrents of devices were enhanced in the presence of an optimal amount of the 1,3,4-oxadiazole moieties, thereby leading to improved power conversion efficiencies. The photovoltaic device based on the copolymer P15 and PCBM exhibited a PCE of 2.50% under AM 1.5 illumination (100 mW cm–2). The EQE of the device incorporating this polythiophene presenting side chain–tethered 1,3,4-oxadiazole units was greater than that of the device
incorporating low-molecular-weight poly(3-hexylthiophene); as a result, its short circuit current density was also much higher.
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著作目錄
1. Chia-Hung Chou, So-Lin Hsu, Siao-Wei Yeh, Hsu-Shen Wang, Kung-Hwa Wei
“Enhanced Luminance and Thermal Properties of Polyphenylenevinylene Copolymer Presenting Side-Chain-Tethered Silsesquioxane Units” Macromolecules 2005, 38, 9117. (SCI; IF: 4.539)
2. Chia-Hung Chou, Hsu-Shen Wang, Kung-Hwa Wei and Jung Y. Huang,
“Thiophenol-modified CdS nanoparticles enhance the luminescence of benzoxyl dendron-substituted polyfluorene copolymers,” Advanced Functional Materials 2006, 16, 909, (SCI; IF: 6.990)
3. Hsu-Shen Wang, Li-Hua Lin, Shih-Yung Chen, Yuh-Lin Wang,and Kung-Hwa Wei,
“Ordered Polythiophene/Fullerene Composite Core–Shell Nanorod Arrays for Solar Cell Applications”, Nanotechnology, 2009 20, 075201. (SCI; IF: 3.137)
4. Hsu-ShenWang, Shih-Yung Chen, Ming-Hsin Su,Yuh-LinWangand Kung-HwaWei, “Inverted Heterojunction Solar Cells Incorporating Fullerene/
Polythiophene Composite Core/Shell Nanorod Arrays“, Nanotechnology, 2010 21, 145203. (SCI; IF: 3.137)
5. Hsu-Shen Wang, Ming-Shin Su, and Kung-Hwa Wei, “Synthesis and
Characterization of Donor–Acceptor Poly(3-hexylthiophene) Copolymers Presenting 1,3,4-Oxadiazole Units and Their Application to Photovoltaic Cells“, Journal of Polymer Science Part A: Polymer Chemistry, 2010 48, 3331. (SCI; IF: 3.971)
6. Hsu-Shen Wang, Shih-Yung Chen, Yuh-Lin Wang, and Kung-Hwa Wei,
“Nanostructured Arrays Presenting TiO2 nanorods/ Poly(3-hexylthiophene) for Solar Cells Application“, Journal of Nanoscience and Nanotechnology, 2010 accepted. (SCI;
IF: 1.435)
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學經歷資料
原子力顯微鏡(AFM; conducting,tapping,contact mode，DI Multimode 管理者，
D3100 )、穿透式電子顯微鏡(TEM，JEOL 2010，FEI Spirit TWIN 120 keV)、掃 描式電子顯微鏡(SEM，JEOL 6500，JEOL 6700)、核磁共振光譜儀(Varian NMR and Brucker NMR)、 微差掃描卡計(DSC)、熱重量分析儀(TGA)、質譜儀(Mass)、凝