Dislocation-Mediated Quantum Melting
Aron Beekman
Department of Physics & Research and Education Center for Natural Sciences Keio University (Hiyoshi, Yokohama)
aron@phys-h.keio.ac.jp
“Chiral Matter and Topology” workshop, NTU, December 7th 2018
supported by:
• MEXT-Supported Program for the Strategic Research Foundation at Private Universities
“Topological Science” (grant no. S1511006)
• JSPS Kakenhi Grant-in-Aid for Early-Career Scientists (grant no. 18K13502)
Dislocation-Mediated Quantum Melting
Aron Beekman
Department of Physics & Research and Education Center for Natural Sciences Keio University (Hiyoshi, Yokohama)
aron@phys-h.keio.ac.jp
“Chiral Matter and Topology” workshop, NTU, December 7th 2018
supported by:
• MEXT-Supported Program for the Strategic Research Foundation at Private Universities
“Topological Science” (grant no. S1511006)
• JSPS Kakenhi Grant-in-Aid for Early-Career Scientists (grant no. 18K13502)
Dislocation-Mediated Quantum Melting
Aron Beekman
Department of Physics & Research and Education Center for Natural Sciences Keio University (Hiyoshi, Yokohama)
aron@phys-h.keio.ac.jp
“Chiral Matter and Topology” workshop, NTU, December 7th 2018
supported by:
• MEXT-Supported Program for the Strategic Research Foundation at Private Universities
“Topological Science” (grant no. S1511006)
• JSPS Kakenhi Grant-in-Aid for Early-Career Scientists (grant no. 18K13502) Nematic
Isotropic Smectic
Crystal
Figure 3 Schematic view of the local stripe order in the various phases discussed in the text. Here, we have assumed that the stripes maintain their integrity throughout, although in reality they must certainly become less and less well def ned as the system becomes increasingly quantum, until eventually they are not the correct variables for describing the important correlations in the system.
Heavy lines represent liquid-like stripes, along which the electrons can f ow, whereas the f lled circles representpinned, density-wave order along the stripes.
The stripes are shown executing more or less harmonic oscillations in the smectic phase. Two dislocations, which play an essential role in the smectic-to- nematic phase transition, are shown in the view of the nematic phase.
Dislocations
Topological defect associated with translational order
Topological charge: Burgers vector Ba
Outline
• Classical dislocations
• restricted motion
• interdependence with disclinations
• Dislocation condensation = quantum melting
• duality
• deconfinement of disclinations
• Recent developments
• critical properties of dislocation condensation
• relation to fractons
• superfluids without U (1) breaking
Aron Beekman Dislocation-Mediated Quantum Melting 2 / 21
Dislocation motion
(a) initial dislocation (b) glide motion (c) climb motion
climb motion involves the addition/removal of (interstitial) particles and is suppressed ↔ particle number conservation
Glide constraint:
“dislocations can only move in the direction of their Burgers vector”
Dislocations and disclinations
(d) dislocation (e) disclination (f) Volterra construction
• dislocation : Burgers vector Ba, torsion
• disclination : Frank scalar Ω, curvature
Aron Beekman Dislocation-Mediated Quantum Melting 4 / 21
Interdependence of dislocations and disclinations
(g) atoms (h) disclination (i) stack of dislocations
(j) disclination pair (k) two disclination pairs
Defect-mediated melting
Nobel Prize in Physics 2016 citation :
‘‘for theoretical discoveries of topological phase transitions ...”
Berezinshkii–Kosterlitz–Thouless melting
Berezinskii 1970-71; Kosterlitz Thouless 1972-73
• in 2D, no true long-range order
• higher dimensions: order–disorder defect-unbinding phase transition
• 2+1D superfluid–Bose-Mott insulator quantum phase transition
Aron Beekman Dislocation-Mediated Quantum Melting 6 / 21
Defect-mediated melting
Nobel Prize in Physics 2016 citation :
‘‘for theoretical discoveries of topological phase transitions ...”
Berezinshkii–Kosterlitz–Thouless melting
Berezinskii 1970-71; Kosterlitz Thouless 1972-73
• in 2D, no true long-range order
• higher dimensions: order–disorder defect-unbinding phase transition
• 2+1D superfluid–Bose-Mott insulator quantum phase transition
Going quantum
• D-dim. quantum field theory ↔ D + 1-dim. statistical physics, e.g. 2D superfluid–insulator QPT is in the 3D XY universality class.
• Time axis is the additional dimension. Statistical physics of worldlines.
Aron Beekman Dislocation-Mediated Quantum Melting 7 / 21
Two-dimensional classical melting
• Unbinding of dislocations = loss of translational order
Berezinskii 1970-71; Kosterlitz Thouless 1972-73
• Two types of topological defects
(a) dislocation – translational (b) disclination – rotational
Nelson Halperin 1978-79; Young 1979
Two-dimensional classical melting
• Unbinding of dislocations = loss of translational order
Berezinskii 1970-71; Kosterlitz Thouless 1972-73
• Two types of topological defects
(a) dislocation – translational (b) disclination – rotational
Nelson Halperin 1978-79; Young 1979
Aron Beekman Dislocation-Mediated Quantum Melting 8 / 21
Two-dimensional classical melting
• Unbinding of dislocations = loss of translational order
Berezinskii 1970-71; Kosterlitz Thouless 1972-73
• Two types of topological defects
(a) dislocation – translational (b) disclination – rotational
Nelson Halperin 1978-79; Young 1979
Two-dimensional classical melting
• Why is the ordinary solid-to-liquid transition first order?
• Simultaneous unbinding
Kleinert 1983
• Towards quantum melting, zero-temperature phase transition
Aron Beekman Dislocation-Mediated Quantum Melting 9 / 21
Two-dimensional classical melting
• Why is the ordinary solid-to-liquid transition first order?
• Simultaneous unbinding
Kleinert 1983
• Towards quantum melting, zero-temperature phase transition
Two-dimensional classical melting
• Why is the ordinary solid-to-liquid transition first order?
• Simultaneous unbinding
Kleinert 1983
• Towards quantum melting, zero-temperature phase transition
Aron Beekman Dislocation-Mediated Quantum Melting 9 / 21
Two-dimensional quantum melting
(a) 2D bound pairs (b) 2D unbound
(c) 2+1D bound loops (d) 2D unbound worldlines
Two-dimensional quantum melting
(a) 2D bound pairs (b) 2D unbound
(c) 2+1D bound loops (d) 2D unbound worldlines
Aron Beekman Dislocation-Mediated Quantum Melting 10 / 21
2+1D dislocation-mediated quantum melting
• ‘Statistical physics’/quantum partition sum of dislocation worldlines
• Role of inverse temperature is played by temporal correlations
• 2D quantum corresponds to 3D classical
• Proliferation of dislocation lines 3D classical
Kleinert 1980s
• Time direction manifestly different from space directions
• Condensation of dislocations = proliferation of worldlines 2+1D quantum
Zaanen Nussinov Mukhin 2004; Cvetkovic Zaanen 2006; AJB et al. 2017
Essence: the dislocation condensate is decribed by a collective complex field Ψa(x), a = x, y, |Ψa|2∼ density of ‘worldline tangle’ (1)
Ginzburg–Landau-type action LGL= X
a=x,y
1
2αa|Ψa|2+1 4βa|Ψa|4
+1
2γ|Ψx|2|Ψy|2 (2)
2+1D dislocation-mediated quantum melting
• ‘Statistical physics’/quantum partition sum of dislocation worldlines
• Role of inverse temperature is played by temporal correlations
• 2D quantum corresponds to 3D classical
• Proliferation of dislocation lines 3D classical
Kleinert 1980s
• Time direction manifestly different from space directions
• Condensation of dislocations = proliferation of worldlines 2+1D quantum
Zaanen Nussinov Mukhin 2004; Cvetkovic Zaanen 2006; AJB et al. 2017
Essence: the dislocation condensate is decribed by a collective complex field Ψa(x), a = x, y, |Ψa|2∼ density of ‘worldline tangle’ (1)
Ginzburg–Landau-type action LGL= X
a=x,y
1
2αa|Ψa|2+1 4βa|Ψa|4
+1
2γ|Ψx|2|Ψy|2 (2)
Aron Beekman Dislocation-Mediated Quantum Melting 11 / 21
Dual gauge field theory of defect-mediated melting
• Duality mapping, analogous to vortex–boson / Abelian-Higgs duality
• Phonons are gauge bosons orstress photons
• Dislocations areshear stress charges
• A solid is astress vacuumorCoulomb gas of stress charges
• An hexatic is astress superconductor
• Dual Meissner effect: shear stress is expelled from the liquid crystal
Dual gauge field theory of defect-mediated melting
• Duality mapping, analogous to vortex–boson / Abelian-Higgs duality
• Phonons are gauge bosons orstress photons
• Dislocations areshear stress charges
• A solid is astress vacuumorCoulomb gas of stress charges
• An hexatic is astress superconductor
• Dual Meissner effect: shear stress is expelled from the liquid crystal
Aron Beekman Dislocation-Mediated Quantum Melting 12 / 21
Dual gauge field theory of defect-mediated melting
• Duality mapping, analogous to vortex–boson / Abelian-Higgs duality
• Phonons are gauge bosons orstress photons
• Dislocations areshear stress charges
• A solid is astress vacuumorCoulomb gas of stress charges
• An hexatic is astress superconductor
• Dual Meissner effect: shear stress is expelled from the liquid crystal
Dual stress effective action
Classical stress energy Esolid= 12σam Cmnab−1
| {z }
elastic moduli
σbn
Quantum stress Lagrangian Lsolid=2ρ1(στa)2+12σamCmnab−1 σbn
Lsolid= 1
2(µκλ∂κbaλ)Cµνab−1 (νρσ∂ρbaσ), LGL= X
a=x,y
1
2αa|Ψa|2+1 4βa|Ψa|4
+1
2γ|Ψx|2|Ψy|2, Lcoupling= 1
2 X
a=x,y
|(∂µ− ibaµ− iλτ µa)Ψa|2.
Aron Beekman Dislocation-Mediated Quantum Melting 13 / 21
Dual stress effective action
Classical stress energy Esolid= 12σam Cmnab−1
| {z }
elastic moduli
σbn
Quantum stress Lagrangian Lsolid=2ρ1(στa)2+12σamCmnab−1 σbn
Stress is conserved ∂τστa+ ∂mσma = ∂µσµa= 0 Dual stress gauge field σµa= µνλ∂νbaλ, a = x, y
Lsolid= 1
2(µκλ∂κbaλ)Cµνab−1 (νρσ∂ρbaσ), LGL= X
a=x,y
1
2αa|Ψa|2+1 4βa|Ψa|4
+1
2γ|Ψx|2|Ψy|2, Lcoupling= 1
2 X
a=x,y
|(∂µ− ibaµ− iλτ µa)Ψa|2.
Dual stress effective action
Classical stress energy Esolid= 12σam Cmnab−1
| {z }
elastic moduli
σbn
Quantum stress Lagrangian Lsolid=2ρ1(στa)2+12σamCmnab−1 σbn
Stress is conserved ∂τστa+ ∂mσma = ∂µσµa= 0 Dual stress gauge field σµa= µνλ∂νbaλ, a = x, y
Lsolid= 1
2(µκλ∂κbaλ)Cµνab−1 (νρσ∂ρbaσ),
LGL= X
a=x,y
1
2αa|Ψa|2+1 4βa|Ψa|4
+1
2γ|Ψx|2|Ψy|2, Lcoupling= 1
2 X
a=x,y
|(∂µ− ibaµ− iλτ µa)Ψa|2.
Aron Beekman Dislocation-Mediated Quantum Melting 13 / 21
Dual stress effective action
Classical stress energy Esolid= 12σam Cmnab−1
| {z }
elastic moduli
σbn
Quantum stress Lagrangian Lsolid=2ρ1(στa)2+12σamCmnab−1 σbn
Stress is conserved ∂τστa+ ∂mσma = ∂µσµa= 0 Dual stress gauge field σµa= µνλ∂νbaλ, a = x, y
Lsolid= 1
2(µκλ∂κbaλ)Cµνab−1 (νρσ∂ρbaσ), LGL= X
a=x,y
1
2αa|Ψa|2+1 4βa|Ψa|4
+1
2γ|Ψx|2|Ψy|2, Lcoupling= 1
2 X
a=x,y
|(∂µ− ibaµ− iλτ µa)Ψa|2.
Main results
1 Phonons are gauge bosons
2 The disordered solid is a stress superconductor
3 The disordered solid is a real superfluid(longitudinal response)
4 Rotational Goldstone mode deconfines in qu. hexatic(transverse response) 5 Transverse phonon becomes gapped shear mode in quantum hexatic 6 The gapped shear mode is detectable by finite-momentum spectroscopy
AJB et al. Phys. Rep. 683, 1 (2017)
stress vacuum stress superconductor
dislocations unbound dislocations bound torque vacuum torque confined torque superconductor
disclinations bound disclinations confined disclinations unbound
solid superfluid quantum hexatic
ρ
longitudinal transverse
phonon phase mode
phase mode
rotational NG mode phonon response
Aron Beekman Dislocation-Mediated Quantum Melting 14 / 21
Disclination deconfinement
• Displacement field ua(x)
• Rotation field ωab= ∂aub(x) − ∂bua(x)
solid hexatic
Lagrangian stress ua(∂t2+ ∇2)ua ua(∂t2+ ∇2+ |Ψ|2)ua rotation ωab∇2(∂t2+ ∇2)ωab . . . + ωab|Ψ|2(∂2t + ∇2)ωab propagator stress ω2+q1 2 ω2+q21+|Ψ|2
rotation q2(ω21+q2)
. . . +
ω|Ψ|2+q22 static limit stress 1q2
1 q2+|Ψ|2 rotation q14
. . . +
|Ψ|q22For the same reason, rotational Nambu–Goldstone modes are absent in solid, but present in quantum hexatic.
Helium monolayer experiments
Helium monolayers on ZYX exfoliated graphite S. Nakamura et al. PRB 94, 180501(R) (2016)
Aron Beekman Dislocation-Mediated Quantum Melting 16 / 21
Helium monolayer experiments
Helium monolayers on ZYX exfoliated graphite S. Nakamura et al. PRB 94, 180501(R) (2016)
• anomaly in specific heat : BKT-like defect-unbinding transition
Helium monolayer experiments
Helium monolayers on ZYX exfoliated graphite S. Nakamura et al. PRB 94, 180501(R) (2016)
• anomaly in specific heat : BKT-like defect-unbinding transition
• three separate peaks
Aron Beekman Dislocation-Mediated Quantum Melting 16 / 21
Helium monolayer experiments
Helium monolayers on ZYX exfoliated graphite S. Nakamura et al. PRB 94, 180501(R) (2016)
• anomaly in specific heat : BKT-like defect-unbinding transition
• three separate peaks
Helium monolayer experiments
Helium monolayers on ZYX exfoliated graphite S. Nakamura et al. PRB 94, 180501(R) (2016)
• anomaly in specific heat : BKT-like defect-unbinding transition
• three separate peaks
Aron Beekman Dislocation-Mediated Quantum Melting 16 / 21
Critical properties of solid-to-hexatic quantum melting
Effective field theory (Ginzburg–Landau) Lsolid= 1
2(µκλ∂κbaλ)Cµνab−1 (νρσ∂ρbaσ), LGL= X
a=x,y
1
2αa|Ψa|2+1 4βa|Ψa|4
+1
2γ|Ψx|2|Ψy|2, Lcoupling= 1
2 X
a=x,y
|(∂µ− ibaµ− iλτ µa)Ψa|2. Simplified to
Lsolid=1
2(∇ × bx)2+1
2(∇ × by)2, LGL=1
2m2(|Ψx|2+ |Ψy|2) +1
4λ(|Ψx|4+ |Ψy|4) +1
2g|Ψx|2|Ψy|2, Lcoupling =1
2|(∇ − iebx)Ψx|2+1
2|(∇ − iebx)Ψy|2
• Onlym2 andλ2: O(2) Wilson-Fisher theory
• withe: charged O(2), Abelian-Higgs model
• withg: O(2) × O(2), two-component BEC
Critical properties of solid-to-hexatic quantum melting in d = 3
Abelian-Higgs d = 3
shown with FRG down to N = 2:
G. Fejos & T. Hatsuda
PRD 93, 121702 (2016) 96, 056018 (2017)
Two-component BEC d = 3
ε-expansion Ceccarelli et al.
PRA 92, 024513 (2016) 93, 033647 (2017)
Work in progress (with Gergely Fejos):
• FRG for charged O(2) × O(2) in d = 3, charged fixed points
• Influence of stress gauge field dynamics
• Influence of glide constraint
• Quantum critical exponent for specific heat
Aron Beekman Dislocation-Mediated Quantum Melting 18 / 21
Relation to fracton physics
Fractons: objects/particles with spatially restricted dynamics
Superfluid sound
“Superfluid Goldstone mode arises only when U (1) particle conservation symmetry is broken, i.e. when the glide constraint is relaxed.”
Pretko & Radzihovsky arXiv:1808.05616 Kumar & Potter arXiv:1808.05621
Redundant Goldstone modes: Superfluid breaks boosts and particle conservation. Solid breaks boosts, translations and rotations.
Nicolis, Brauner, Watanabe, Hidaka, . . .
Aron Beekman Dislocation-Mediated Quantum Melting 20 / 21
Superfluid sound
“Superfluid Goldstone mode arises only when U (1) particle conservation symmetry is broken, i.e. when the glide constraint is relaxed.”
Pretko & Radzihovsky arXiv:1808.05616 Kumar & Potter arXiv:1808.05621
Redundant Goldstone modes: Superfluid breaks boosts and particle conservation. Solid breaks boosts, translations and rotations.
Nicolis, Brauner, Watanabe, Hidaka, . . .
Summary
• Condensation of topological defects as symmetry-restoring phase transition
• Topological defects in solids study case for restricted mobility
• dislocations: glide constraint
• disclination: confinement
• Possibly novel critical behaviour
• Nature of superfluid sound
Collaborators:
Jan Zaanen Leiden Robert-Jan Slager Dresden Jaakko Nissinen Aalto Vladimir Cvetkovic
Kai Wu Zohar Nussinov St. Louis
Ke Liu Munich Gergely Fejos Keio U
Aron Beekman Dislocation-Mediated Quantum Melting 21 / 21
Assumptions and limitations
• Zero temperature
• Ginzburg–Landau → only near the phase transition
• London limit, phase fluctuations only
• Maximal crystalline correlations (collective physics only)
• No interstitials
• No disclinations
• Bosons onlybut 4-He and 3-He experiments similar
• Isotropic solid only
3D quantum liquid crystals
t x y
µ
dislocation worldline
t x y
ν µ
dislocation worldsheet
• phonons are now two-form gauge fields bµν
• quantum versions of columnar, smectic and nematic liquid crystals
Goldstone modes phonons
rotational
solid columnar smectic nematic
2+1D 2/0 – 1/0 0/1
3+1D 3/0 2/0 1/1 0/3
AJB, J. Nissinen, K. Wu, J. Zaanen, Physical Review B 96, 165115 (2017)